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Don't expect much beauty using cartoon/storybook shaders on sprite and mixed sprite/3D games. FF7, FF8..., ChronoCross have their moments with them but would need a different from-the-begining texture handling for something called at least acceptable.
They (Cartoon, Storybook shaders) are fast enough for anything with a 3DMark2003 score of 5000 or higher.
Currently some games can IMO look nice with them, for example Spyro the dragon or Crash bandicoot etc.
What matters the most is the native PSX game resolution.
For the combined sprite/3D 320x240 games i reccomend something with an AA touch (AA shader, Natural vision shader).
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